同位素分析儀-甲醛分析儀-北京世紀朝陽科技發展有限公司

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測量應用案例-20210102

2021-01-13 10:11:38

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文獻名: Ultrathin Co-Co LDHs nanosheets assembled vertically on MXene: 3D nanoarrays for boosted visible-light-driven CO2 reduction

 

作者: Weiyi Chenab; Bin Hanab; Yili Xieab; Shujie Liangab; Hong Dengab; Zhang Linab

aSchool of Environment and Energy, Key Laboratory of Pollution Control and Ecosystem Restoration in Industry Clusters (Ministry of Education), South China University of Technology, Guangzhou 510006, China

bGuangdong Engineering and Technology Research Center for Environmental Nanomaterials, South China University of Technology, Guangzhou 510006, China

 

摘要:Converting carbon dioxide (CO2) to multiple energy-rich chemicals by photocatalysis could validly mitigate the severe issues of climate changes and energy shortages. Exploring efficient catalysts for enhancing the performance of CO2 photoreduction is still challenging. Herein, a novel three-dimensional hierarchical Co-Co layered double hydroxide/Ti3C2TX nanosheets (Co-Co LDH/TNS) nanoarray was successfully prepared via an in-situ MOF-derived strategy. This wise design rationally integrates the functional and structural merits of active Co species with conductive MXene to a hierarchical nanoarray architecture composed of ultrathin nanosheets, which can remarkably promote separation of photogenerated charge carriers and accelerate electrons transmission. Benefitting from these features, the hierarchical Co-Co LDH/TNS composites manifest significant enhancement on the CO2-to-CO evolving rate (1.25 × 104 μmol h?1 g?1) under illumination (>400 nm) with a high apparent quantum efficiency (0.92%) and excellent stability. Our work demonstrates that 3D hybrid structure composed of MXene species can serve as promising candidates for CO2 photoreduction, providing fundamental guidance to improve photocatalytic performance by rational engineering of complex hierarchical architecture materials.


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同位素分析儀-甲醛分析儀-北京世紀朝陽科技發展有限公司 同位素分析儀-甲醛分析儀-北京世紀朝陽科技發展有限公司
同位素分析儀-甲醛分析儀-北京世紀朝陽科技發展有限公司
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